title: Operando magnetic resonance: monitoring the evolution of conversion and product distribution during the heterogeneous catalytic ethene oligomerisation reaction.
abstract: Operando magnetic resonance (MR) spectroscopy has been used to follow an ethene oligomerisation reaction performed at 110 °C, 28 barg over a 1 wt% Ni/SiO2-Al2O3 catalyst. Spectra acquired over the timecourse of the reaction allow the calculation of conversion and product distribution as a function of time-on-stream.
authors.affiliation: Department of Chemical Engineering and Biotechnology, University of Cambridge, Pembroke Street, Cambridge, CB2 3RA, UK. lfg1@cam.ac.uk.
authors.forename: S Tegan
authors.initials: ST
authors.lastname: Roberts
authors.forename: Matthew P
authors.initials: MP
authors.lastname: Renshaw
authors.forename: Michal
authors.initials: M
authors.lastname: Lutecki
authors.forename: James
authors.initials: J
authors.lastname: McGregor
authors.forename: Andrew J
authors.initials: AJ
authors.lastname: Sederman
authors.forename: Mick D
authors.initials: MD
authors.lastname: Mantle
authors.forename: Lynn F
authors.initials: LF
authors.lastname: Gladden