title: Bonner sphere measurements of 241Am-B and 241Am-F neutron energy spectra unfolded using high-resolution a priori data.
abstract: High-resolution neutron energy spectra, covering the entire energy range of interest, for two standard radionuclide neutron sources ((241)Am-B and (241)Am-F) have been derived from Bonner sphere measurements by using high-resolution a priori data in the unfolding process. In each case, two a priori spectra were used, one from a two-stage calculation and also one from a combination of the calculated spectrum with a high-resolution measured spectrum. The unfolded spectra are compared with those published elsewhere and show significant differences from the ISO- and IAEA-recommended spectra for (241)Am-B and (241)Am-F, respectively. Values for the fluence-average energy and fluence-to-dose-equivalent conversion coefficients are presented for the new spectra, and the implications of the new spectra for the emission rates of the sources when measured by the manganese bath technique are also determined.
authors.affiliation: National Physical Laboratory, Hampton Road, Teddington, Middx TW11 0LW, UK neil.roberts@npl.co.uk.
authors.forename: N J
authors.initials: NJ
authors.lastname: Roberts
authors.affiliation: National Physical Laboratory, Hampton Road, Teddington, Middx TW11 0LW, UK.
authors.forename: L N
authors.initials: LN
authors.lastname: Jones
authors.affiliation: National Physical Laboratory, Hampton Road, Teddington, Middx TW11 0LW, UK.
authors.forename: Z Z
authors.initials: ZZ
authors.lastname: Liu
authors.affiliation: National Physical Laboratory, Hampton Road, Teddington, Middx TW11 0LW, UK.
authors.forename: H
authors.initials: H
authors.lastname: Tagziria
authors.affiliation: National Physical Laboratory, Hampton Road, Teddington, Middx TW11 0LW, UK.
authors.forename: D J
authors.initials: DJ
authors.lastname: Thomas
mesh_terms: D000465:Algorithms; D000576:Americium / Q000737:chemistry*; D001895:Boron / Q000737:chemistry*; D003198:Computer Simulation; D004867:Equipment Design; D005459:Fluorides / Q000737:chemistry*; D006371:Helium; D007477:Ions; D008345:Manganese / Q000737:chemistry; D009010:Monte Carlo Method; D009502:Neutrons; D020959:Polyethylene / Q000737:chemistry; D011829:Radiation Dosage; D011834:Radiation Monitoring / Q000295:instrumentation* / Q000379:methods; D011835:Radiation Protection / Q000379:methods; D011868:Radioisotopes / Q000032:analysis; D013053:Spectrophotometry
chemical_list: D007477:Ions; D011868:Radioisotopes; D006371:Helium; D008345:Manganese; D020959:Polyethylene; D001895:Boron; D005459:Fluorides; D000576:Americium