title: Plutonium in soils from northeast China and its potential application for evaluation of soil erosion.
abstract: Surface and soil core samples from northeast China were analyzed for Pu isotopes. The measured (240)Pu/(239)Pu atomic ratios and (239 + 240)Pu/(137)Cs activity ratios revealed that the global fallout is the dominant source of Pu and (137)Cs at these sites. Migration behavior of Pu varying with land type and human activities resulted in different distribution of Pu in surface soils. A sub-surface maximum followed by exponential decline of (239 + 240)Pu concentrations was observed in an undisturbed soil core, with a total (239 + 240)Pu inventory of 86.9 Bq/m(2) and more than 85% accumulated in 0 ~ 20 cm layers. While only half inventory of Pu was obtained in another soil core and no sub-surface maximum value occurred. Erosion of topsoil in the site should be the most possible reason for the significantly lower Pu inventory, which is also supported by the reported (137)Cs profiles. These results demonstrated that Pu could be applied as an ideal substitute of (137)Cs for soil erosion study in the future.
authors: 1] The Key Laboratory of Coastal and Island Development of Ministry of Education, Nanjing University, Nanjing 210093, China [2] Center for Nuclear Technologies, Technical University of Denmark, Risø Campus, Roskilde 4000, Denmark.
authors: Yihong
authors: Y
authors: Xu
authors: Center for Nuclear Technologies, Technical University of Denmark, Risø Campus, Roskilde 4000, Denmark.
authors: Jixin
authors: J
authors: Qiao
authors: 1] Center for Nuclear Technologies, Technical University of Denmark, Risø Campus, Roskilde 4000, Denmark [2] Xi'an AMS Center, SKLLQG, Institute of Earth Environment, CAS, Xi'an 710075, China.
authors: Xiaolin
authors: X
authors: Hou
authors: The Key Laboratory of Coastal and Island Development of Ministry of Education, Nanjing University, Nanjing 210093, China.
authors: Shaoming
authors: S
authors: Pan