title: Occurrence and fate of perfluoroalkyl substances in marine sediments from the Chinese Bohai Sea, Yellow Sea, and East China Sea.
abstract: In this study, 166 surface sediments and 3 sediment cores from the Bohai Sea (BS), Yellow Sea (YS) and East China Sea (ECS) in China were collected to investigate the spatial and temporal distributions and the transport of PFASs. PFASs concentrations in the surface sediments ranged from below detection limit (<LOD) to 2.78 ng g(-1) with an average value of 0.55 ng g(-1) on a dry weight basis (dw). A general decreasing trend of PFASs from the coast areas to the open sea was found. Multivariate regression analysis indicated pH and longitude were the major factors influencing surficial distributions of PFASs in the sampling areas (R(2) = 0.29, p < 0.01). Total PFASs concentrations in the sediment cores ranged from <LOD to 1.65 ng g(-1) dw, with an increasing trend from the lower to the upper layers, corresponding well to the increasing production and usage in China in recent years.
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Yan
authors.initials: Y
authors.lastname: Gao
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Jianjie
authors.initials: J
authors.lastname: Fu
authors.affiliation: School of Chemistry and Chemical Engineering, University of Chinese Academy of Sciences, Beijing 100049, China.
authors.forename: Lixi
authors.initials: L
authors.lastname: Zeng
authors.affiliation: School of Public Health, University of Illinois at Chicago, Chicago, USA.
authors.forename: An
authors.initials: A
authors.lastname: Li
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Huijuan
authors.initials: H
authors.lastname: Li
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Nali
authors.initials: N
authors.lastname: Zhu
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Runzeng
authors.initials: R
authors.lastname: Liu
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Aifeng
authors.initials: A
authors.lastname: Liu
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China. Electronic address: ywwang@rcees.ac.cn.
authors.forename: Yawei
authors.initials: Y
authors.lastname: Wang
authors.affiliation: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, P.O. Box 2871, Beijing 100085, China.
authors.forename: Guibin
authors.initials: G
authors.lastname: Jiang
mesh_terms: D002681:China; D004784:Environmental Monitoring; D005466:Fluorocarbons / Q000032:analysis*; D019015:Geologic Sediments / Q000737:chemistry*; D009792:Oceans and Seas; D014874:Water Pollutants, Chemical / Q000032:analysis*
chemical_list: D005466:Fluorocarbons; D014874:Water Pollutants, Chemical
keywords: Marine sediment; Perfluoroalkyl substances; Spatial distribution; Temporal distribution