title: Laser spark ignition of premixed methane-air mixtures: parameter measurements and determination of key factors for ultimate ignition results.
abstract: In this study, we present an experimental investigation of the parameters of the laser spark ignition of premixed methane-air mixtures and the determination of the key factors for the ultimate ignition result. Ignition is achieved in a mesh honeycomb burner using the 1064 nm output of a neodymium-doped yttrium aluminum garnet (Nd : YAG) laser. All pertinent laser ignition parameters, including the minimum ignition energy, the ignition time and blow out time, and the effects that the variation of experimental conditions, such as the spark energy, ignition position, equivalence ratio (ER), and flow rate, have on these parameters have been addressed systematically. To identify the key factors for the ultimate result of laser ignition, several parameters of the ignition processes are measured simultaneously, with an emphasis given to the temporal behavior of the hydroxyl (OH) radicals in relation to the data regarding the spark energy and the local ER. A clear finding of the study is that successful ignition events are always related to higher OH radical photon emissions, considered to be proportional to the concentration level of the OH radicals present, thus indicating a direct link between the OH level at early times (on a microsecond scale) and the ultimate result of laser ignition. Two-dimensional correlation plots of the spark energy, local ER, and OH radical photon count at early times with the ultimate results of laser ignition indicate that the spark energy and local ER do not play a critical role in determining the success or failure of the ignition and that the OH concentration in the early time range is the key factor in determining the final fate of laser ignition. Finally, on the basis of the results obtained here and in the existing literature, some considerations of the mechanism of laser ignition are presented.
authors.affiliation: Harbin Institute of Technology, National Key Laboratory of Science and Technology on Tunable Laser, Harbin, Heilongjiang 150080, China.
authors.forename: Xiaohui
authors.initials: X
authors.lastname: Li
authors.forename: Benjamin W
authors.initials: BW
authors.lastname: Smith
authors.forename: Nicoló
authors.initials: N
authors.lastname: Omenetto