title: The impacts of summer monsoons on the ozone budget of the atmospheric boundary layer of the Asia-Pacific region.
abstract: The seasonal and inter-annual variations of ozone (O3) in the atmospheric boundary layer of the Asia-Pacific Ocean were investigated using model simulations (2001-2007) from the Model of Ozone and Related chemical Tracers, version 4 (MOZART-4). The simulated O3 and diagnostic precipitation are in good agreement with the observations. Model results suggest that the Asia-Pacific monsoon significantly influences the seasonal and inter-annual variations of ozone. The differences of anthropogenic emissions and zonal winds in meridional directions cause a pollutants' transition zone at approximately 20°-30°N. The onset of summer monsoons with a northward migration of the rain belt leads the transition zone to drift north, eventually causing a summer minimum of ozone to the north of 30°N. In years with an early onset of summer monsoons, strong inflows of clean oceanic air lead to low ozone at polluted oceanic sites near the continent, while strong outflows from the continent exist, resulting in high levels of O3 over remote portions of the Asia-Pacific Ocean. The reverse is true in years when the summer monsoon onset is late.
authors.affiliation: Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing 210044, China; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science and Technology, Nanjing 210044, China.
authors.forename: Xuewei
authors.initials: X
authors.lastname: Hou
authors.affiliation: Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing 210044, China; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science and Technology, Nanjing 210044, China. Electronic address: binzhu@nuist.edu.cn.
authors.forename: Bin
authors.initials: B
authors.lastname: Zhu
authors.affiliation: Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing 210044, China.
authors.forename: Dongdong
authors.initials: D
authors.lastname: Fei
authors.affiliation: Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters, Nanjing University of Information Science & Technology, Nanjing 210044, China; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science and Technology, Nanjing 210044, China.
authors.forename: Dongdong
authors.initials: D
authors.lastname: Wang
mesh_terms: D000393:Air Pollutants / Q000032:analysis*; D000397:Air Pollution / Q000706:statistics & numerical data; D001208:Asia; D001272:Atmosphere / Q000737:chemistry; D004784:Environmental Monitoring; D010126:Ozone / Q000032:analysis*; D010140:Pacific Ocean; D012621:Seasons
chemical_list: D000393:Air Pollutants; D010126:Ozone
keywords: Asia-Pacific monsoon; Transition zone; Tropospheric ozone