title: Estimation of the Arctic aerosols from local and long-range transport using relationships between ²¹⁰Pb and ²¹²Pb atmospheric activity concentrations.
abstract: In this study, the aerosol activity concentrations of (210)Pb at 28 Canadian radiological monitoring stations from 2009 to 2013 were analyzed. The results show that the ratio of (210)Pb winter average concentration to summer average concentration increases with increasing latitude. This could be used to evaluate the transport of pollutants to the Arctic region such as the Arctic haze from Eurasia through long-range atmospheric transport during winter. Based on 12 years of monitoring results from the Yellowknife station that includes both (210)Pb and (212)Pb concentrations, the study confirms that the seasonal distribution of (210)Pb to (212)Pb activity concentration ratios has a significant peak in winter and a relatively low value in summer, which can be used as an indicator of the air mass flow to the Arctic. The period dominated by long-range aerosol transport and Arctic haze was estimated by fitting a Gaussian distribution function to the peak values of this ratio in winter. A peak width parameter of full width at half maximum (FWHM) allows a year by year estimate of the period of influence by long-range transport of aerosols, and this varied between 67 and 88 days in this study. The fitted Gaussian peak also shows that the season of the continental influenced air mass in Yellowknife usually starts in mid-to-late November and ends in mid-to-late April. Thus, the (210)Pb to (212)Pb ratio distributions may enable the determination of periods dominated by long-range aerosol transport and the scale of the Arctic haze at different latitudes.
authors.affiliation: Radiation Protection Bureau of Health Canada, 775 Brookfield Road, Ottawa, Ontario K1A 1C1, Canada. Electronic address: weihua.zhang@hc-sc.gc.ca.
authors.forename: Weihua
authors.initials: W
authors.lastname: Zhang
authors.affiliation: Radiation Protection Bureau of Health Canada, 775 Brookfield Road, Ottawa, Ontario K1A 1C1, Canada.
authors.forename: Jing
authors.initials: J
authors.lastname: Chen
authors.affiliation: Radiation Protection Bureau of Health Canada, 775 Brookfield Road, Ottawa, Ontario K1A 1C1, Canada.
authors.forename: Kurt
authors.initials: K
authors.lastname: Ungar
authors.affiliation: Radiation Protection Bureau of Health Canada, 775 Brookfield Road, Ottawa, Ontario K1A 1C1, Canada.
authors.forename: Michael
authors.initials: M
authors.lastname: Cooke
mesh_terms: D000336:Aerosols / Q000032:analysis*; D000392:Air Movements; D000396:Air Pollutants, Radioactive / Q000032:analysis*; D001110:Arctic Regions; D002170:Canada; D007856:Lead Radioisotopes / Q000032:analysis*; D016011:Normal Distribution; D011834:Radiation Monitoring / Q000379:methods*; D012621:Seasons
chemical_list: D000336:Aerosols; D000396:Air Pollutants, Radioactive; D007856:Lead Radioisotopes
keywords: (210)Pb/(212)Pb activity ratios; Aerosol radioactivity monitoring; Local and long-range transport scale; The Arctic haze