title: Spatial distribution and temporal trends of mercury and arsenic in remote timberline coniferous forests, eastern of the Tibet Plateau, China.
abstract: An intensive investigation was conducted to study the spatial distribution and temporal variety trend of mercury and arsenic in plant tissue and soil profile in the eastern of the Tibet Plateau and to explore the possible sources of these two elements. At present, rare information is available on mercury (Hg) and arsenic (As) of timberline forests in the Tibet Plateau. Here, we present preliminary results on these two elements in leaves, twigs, root, litterfall, and soil. Geostatistical analyst of the ArcGIS 10.0 was used to determine the trait of spatial distribution of these two elements. Total arsenic (TAs) mean concentrations in the leaves, twigs, root, litterfall, and A- and C-layer soil ranged from 0.12 mg kg(-1) (n = 60), 0.35 mg kg(-1) (n = 60), 0.48 mg kg(-1) (n = 42), 1.52 mg kg(-1) (n = 84), 16.51 mg kg(-1) (n = 69), and 26.72 mg kg(-1) (n = 69), respectively. Total Hg (THg) mean concentrations in leaves, twigs, root, litterfall, and A- and C-layer soil were 0.0121 mg kg(-1) (n = 60), 0.0078 mg kg(-1) (n = 60), 0.0171 mg kg(-1) (n = 42), 0.0479 mg kg(-1) (n = 84), 0.0852 mg kg(-1) (n = 75), and 0.0251 mg kg(-1) (n = 75), respectively. In general, litterfall trended to accumulate high concentrations of Hg and As. Mercury in the timberline forest showed an increasing trend, whereas arsenic concentrations showed a decreasing trend in A-layer soil and an increasing trend in C-layer soil due to the easy mobile ability of As. Southwest and southeast monsoon could be the influencing factors, and Hg emission from India and China was the possible source of this study area through using a HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) model. It is believed that these observations may offer scientists and policymakers additional understanding of Hg and As concentrations in the remote timberline area, eastern of the Tibet Plateau.
authors: Key Laboratory of Mountain Surface Processes and Ecological Regulation, Institute of Mountain Hazards and Environment, Chinese Academy of Sciences and Ministry of Water Conservancy, Chengdu, China.
authors: Ronggui
authors: R
authors: Tang
authors: Haiming
authors: H
authors: Wang
authors: Ji
authors: J
authors: Luo
authors: Shouqin
authors: S
authors: Sun
authors: Yiwen
authors: Y
authors: Gong
authors: Jia
authors: J
authors: She
authors: Youchao
authors: Y
authors: Chen
authors: Yang
authors: Y
authors: Dandan
authors: Jun
authors: J
authors: Zhou
mesh_terms: D001151:Arsenic / Q000032:analysis*; D004784:Environmental Monitoring; D065928:Forests; D008628:Mercury / Q000032:analysis*; D018515:Plant Leaves / Q000737:chemistry; D018517:Plant Roots / Q000737:chemistry; D012987:Soil / Q000737:chemistry*; D012989:Soil Pollutants / Q000032:analysis; D062211:Spatio-Temporal Analysis; D018609:Tibet; D064028:Tracheophyta
chemical_list: D012987:Soil; D012989:Soil Pollutants; D008628:Mercury; D001151:Arsenic