title: Isotope ratio mass spectrometry as a tool for source inference in forensic science: A critical review.
abstract: Isotope ratio mass spectrometry (IRMS) has been used in numerous fields of forensic science in a source inference perspective. This review compiles the studies published on the application of isotope ratio mass spectrometry (IRMS) to the traditional fields of forensic science so far. It completes the review of Benson et al. [1] and synthesises the extent of knowledge already gathered in the following fields: illicit drugs, flammable liquids, human provenancing, microtraces, explosives and other specific materials (packaging tapes, safety matches, plastics, etc.). For each field, a discussion assesses the state of science and highlights the relevance of the information in a forensic context. Through the different discussions which mark out the review, the potential and limitations of IRMS, as well as the needs and challenges of future studies are emphasized. The paper elicits the various dimensions of the source which can be obtained from the isotope information and demonstrates the transversal nature of IRMS as a tool for source inference.
authors.affiliation: Ecole des Sciences Criminelles, Université de Lausanne, Batochime, 1015 Lausanne-Dorigny, Switzerland. Electronic address: Natacha.Gentile@unil.ch.
authors.forename: Natacha
authors.initials: N
authors.lastname: Gentile
authors.affiliation: Laboratory of Atmospheric Chemistry, Paul Scherrer Institut, 5232 Villigen, Switzerland.
authors.forename: Rolf T W
authors.initials: RT
authors.lastname: Siegwolf
authors.affiliation: Ecole des Sciences Criminelles, Université de Lausanne, Batochime, 1015 Lausanne-Dorigny, Switzerland.
authors.forename: Pierre
authors.initials: P
authors.lastname: Esseiva
authors.affiliation: Linked Forensic Consultants Ltd, Raumati Beach 5255, Wellington, New Zealand.
authors.forename: Sean
authors.initials: S
authors.lastname: Doyle
authors.affiliation: Forensic Science Institute Zurich, 8004 Zurich, Switzerland.
authors.forename: Kurt
authors.initials: K
authors.lastname: Zollinger
authors.affiliation: Ecole des Sciences Criminelles, Université de Lausanne, Batochime, 1015 Lausanne-Dorigny, Switzerland.
authors.forename: Olivier
authors.initials: O
authors.lastname: Delémont
keywords: Discrimination; Forensic; IRMS; Isotope ratio mass spectrometry; Source inference; Stable isotope