title: Photoneutrons from a beryllium reflector: a potential source of problems with Zr-Au flux monitors ink0standardization based neutron activation analysis.
abstract: The assumption that the shape of the epithermal neutron spectrum can be described, in any research reactor, by the 1/E1+αfunction is a fundamental starting point of thek0standardization. This assumption may be questioned from a reactor physics viewpoint. The type of moderator, the existence of neutron reflectors, the additional production of (γ,n) neutrons and resonance capture by construction materials may be different for each reactor, with consequences for the shape of the neutron spectrum. This dependency may explain that various practitioners reported contradicting experiences with the use of Zr-Au flux monitors for the determination of the α-parameter. An objective view on the influence of the design of the reactor and irradiation facility on the shape of the neutron spectrum can be obtained by modeling. This has been applied in the Reactor Institute Delft for reactor configurations in which the irradiation facilities face the fuel elements with the presence of beryllium reflector elements. The Monte Carlo calculations indicate a distortion of the 1/E1+αrelationship at the higher energy edge of the epithermal neutron spectrum. This distortion is attributed to the formation and thermalisation of both photoneutrons and (n, 2n) produced fast neutrons in the beryllium, and has a direct impact on the resonance activation of95Zr, other than represented by the 1/E1+αfunction. The obtained relationship between neutron flux and neutron energy was also used for estimating thef-value and compared with the value obtained by the Delft Cr-Mo-Au flux monitor.
authors.affiliation: Reactor Institute Delft, Delft University of Technology, Mekelweg 15, 2629 JB Delft, The Netherlands.
authors.forename: M J J
authors.initials: MJ
authors.lastname: Koster-Ammerlaan
authors.affiliation: Reactor Institute Delft, Delft University of Technology, Mekelweg 15, 2629 JB Delft, The Netherlands.
authors.forename: P
authors.initials: P
authors.lastname: Bode
authors.affiliation: Reactor Institute Delft, Delft University of Technology, Mekelweg 15, 2629 JB Delft, The Netherlands.
authors.forename: A J M
authors.initials: AJ
authors.lastname: Winkelman
keywords: Bare triple monitor; Cr–Mo–Au monitor; Instrumental neutron activation analysis; Zr–Au monitor; k0-NAA