title: Global deposition and transport efficiencies of radioactive species with respect to modelling credibility after Fukushima (Japan, 2011).
abstract: In this study we conduct a detailed comparison of the modelling response of the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident with global and local observations. We use five different model versions characterized by different horizontal and vertical resolutions of the same General Circulation Model (GCM). Transport efficiencies of (137)Cs across the world are presented as an indication of the expected radioactive impact. Activity concentrations were well represented showing lower Normalized Mean Biases (NMBs) when the better resolved versions of the GCM were used. About 95% of the results using the zoom configuration over Europe (zEur) remained within a factor of 10 from the observations. Close to Japan, the model reproduced well (137)Cs concentrations using the zoom version over Asia (zAsia) showing high correlations, while more than 64% of the modelling results were found within a factor of two from the observations and more than 92% within a factor of 10. Labile and refractory rare radionuclides calculated indirectly showed larger deviations, with about 60% of the simulated concentrations within a factor of 10 from the observations. We estimate that around 23% of the released (137)Cs remained into Japan, while 76% deposited in the oceans. Around 163 TBq deposited over North America, among which 95 TBq over USA, 40 TBq over Canada and 5 TBq over Greenland). About 14 TBq deposited over Europe (mostly in the European part of Russia, Sweden and Norway) and 47 TBq over Asia (mostly in the Asian part of Russia, Philippines and South Korea), while traces were observed over Africa, Oceania and Antarctica. Since the radioactive plume followed a northward direction before its arrival to USA and then to Europe, a significant amount of about 69 TBq deposited in the Arctic, as well. These patterns of deposition are fully consistent with the most recent reports for the accident.
authors.affiliation: CEA-CNRS-UVSQ UMR 8212, IPSL/LSCE (Laboratoire des Sciences du Climat et de l'Environnement), L'Orme des Merisiers, 91191 Gif-sur-Yvette Cedex, France. Electronic address: Nikolaos.Evangeliou@nilu.no.
authors.forename: Nikolaos
authors.initials: N
authors.lastname: Evangeliou
authors.affiliation: CEA-CNRS-UVSQ UMR 8212, IPSL/LSCE (Laboratoire des Sciences du Climat et de l'Environnement), L'Orme des Merisiers, 91191 Gif-sur-Yvette Cedex, France.
authors.forename: Yves
authors.initials: Y
authors.lastname: Balkanski
authors.affiliation: NCSR "Demokritos", Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety (INRASTES), Environmental Radioactivity Laboratory, 15310 Athens, Greece.
authors.forename: Heleni
authors.initials: H
authors.lastname: Florou
authors.affiliation: NCSR "Demokritos", Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety (INRASTES), Environmental Radioactivity Laboratory, 15310 Athens, Greece.
authors.forename: Konstantinos
authors.initials: K
authors.lastname: Eleftheriadis
authors.affiliation: CEA-CNRS-UVSQ UMR 8212, IPSL/LSCE (Laboratoire des Sciences du Climat et de l'Environnement), L'Orme des Merisiers, 91191 Gif-sur-Yvette Cedex, France.
authors.forename: Anne
authors.initials: A
authors.lastname: Cozic
authors.affiliation: NCSR "Demokritos", Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety (INRASTES), Environmental Radioactivity Laboratory, 15310 Athens, Greece.
authors.forename: Panayotis
authors.initials: P
authors.lastname: Kritidis
mesh_terms: D000392:Air Movements; D000396:Air Pollutants, Radioactive / Q000032:analysis*; D002588:Cesium Radioisotopes / Q000032:analysis*; D062406:Fukushima Nuclear Accident; D008962:Models, Theoretical; D011834:Radiation Monitoring / Q000379:methods*; D011847:Radioactive Fallout / Q000032:analysis*
chemical_list: D000396:Air Pollutants, Radioactive; D002588:Cesium Radioisotopes; D011847:Radioactive Fallout
keywords: Accident; Dispersion; Fallout; Radionuclides; Validation