Inelastic Neutron Scattering Investigation in Glassy SiSe2: Complex Dynamics at the Atomic Scale.
A detailed investigation of the THz dynamics in glassy SiSe2 by means of neutron inelastic scattering is presented. To carefully map the translational dynamics and the region of the boson peak, we carried out two different experiments with sharp and broad resolutions coupled with a narrow and a wide kinematic range, respectively. Data show a complex pattern of excitations made up of three components. The most intense one is the prolongation of the longitudinal acoustic mode while two other modes appear in the boson peak region below 3 meV. We propose an interaction model that allows for a consistent identification of the nature of these modes.
Marco
M
Zanatta
‡Dipartimento di Fisica, Università di Trento, I-38050 Povo, Trento, Italy.|¶IPCF CNR, UOS di Roma, c/o Università di Roma ″La Sapienza″, I-00185 Roma, Italy.
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Fontana
∥Institut Laue Langevin, F-38042 Grenoble, France.
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Orecchini
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Petrillo
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Sacchetti
boson peak; chalcogenide; collective dynamics; glasses; vibrational modes