title: Evolution of the surface state in Bi2Se2Te thin films during phase transition.
abstract: Topological insulators, a new quantum state of matter, have created exciting opportunities for studies in topological quantum physics and for exploring spintronics applications due to their gapless helical metallic surface states. In this study, thin films composed of alternate layers of Bi and Se (Te) ({Bi(3 Å)Te(9 Å)}n/{Bi(3 Å)Se(9 Å)}n) were fabricated by controlling the layer thickness within the atomic scale using thermal evaporation techniques. The high-purity growth of uniform Bi2Se2Te1 thin films has not yet been achieved using a thermal evaporation method. However, as a result of a self-ordering process during annealing, an as-grown amorphous film with p-type polarity could transform into single crystalline Bi2Se2Te1 with n-type polarity. Using THz-time domain spectroscopy (THz-TDS) and ultraviolet photoemission spectroscopy (UPS), we concluded that the conductivity is dominated by the Drude contribution, suggesting the presence of a quantum well state and surface states. Moreover we demonstrated that the emission of terahertz waves from the (001) surface of the single crystalline Bi2Se2Te1 thin film would be possible under the excitation of 790 nm femtosecond optical pulses, indicating the presence of a Dirac-fermion, a photo-Dember effect at the surface state and the transient current within the surface depletion region. The results reported herein provide useful information regarding a valuable deposition method that can be useful in studies of the evolution of surface state electrons in topological insulators.
authors: Institute of Physics and Applied Physics, Yonsei University, Seoul 120-749, Korea. mh.cho@yonsei.ac.kr.
authors: Hyejin
authors: H
authors: Choi
authors: Tae Hyeon
authors: TH
authors: Kim
authors: Jimin
authors: J
authors: Chae
authors: Juheyuck
authors: J
authors: Baeck
authors: Chul-Sik
authors: CS
authors: Kee
authors: Kwang-Ho
authors: KH
authors: Jeong
authors: Hong-Sik
authors: HS
authors: Jeong
authors: Chul
authors: C
authors: Kang
authors: Mann-Ho
authors: MH
authors: Cho