title: The Influence of Climate Change on Atmospheric Deposition of Mercury in the Arctic—A Model Sensitivity Study.
abstract: Mercury (Hg) is a global pollutant with adverse health effects on humans and wildlife. It is of special concern in the Arctic due to accumulation in the food web and exposure of the Arctic population through a rich marine diet. Climate change may alter the exposure of the Arctic population to Hg. We have investigated the effect of climate change on the atmospheric Hg transport to and deposition within the Arctic by making a sensitivity study of how the atmospheric chemistry-transport model Danish Eulerian Hemispheric Model (DEHM) reacts to climate change forcing. The total deposition of Hg to the Arctic is 18% lower in the 2090s compared to the 1990s under the applied Special Report on Emissions Scenarios (SRES-A1B) climate scenario. Asia is the major anthropogenic source area (25% of the deposition to the Arctic) followed by Europe (6%) and North America (5%), with the rest arising from the background concentration, and this is independent of the climate. DEHM predicts between a 6% increase (Status Quo scenario) and a 37% decrease (zero anthropogenic emissions scenario) in Hg deposition to the Arctic depending on the applied emission scenario, while the combined effect of future climate and emission changes results in up to 47% lower Hg deposition.
authors.affiliation: Department of Environmental Science and Arctic Research Centre, Aarhus University, Roskilde 4000, Denmark. kmh@envs.au.dk.
authors.forename: Kaj M
authors.initials: KM
authors.lastname: Hansen
authors.affiliation: Department of Environmental Science and Arctic Research Centre, Aarhus University, Roskilde 4000, Denmark. jc@envs.au.dk.
authors.forename: Jesper H
authors.initials: JH
authors.lastname: Christensen
authors.affiliation: Department of Environmental Science and Arctic Research Centre, Aarhus University, Roskilde 4000, Denmark. jbr@envs.au.dk.
authors.forename: Jørgen
authors.initials: J
authors.lastname: Brandt
mesh_terms: D000393:Air Pollutants / Q000032:analysis*; D001110:Arctic Regions; D001272:Atmosphere / Q000737:chemistry*; D057231:Climate Change; D004784:Environmental Monitoring / Q000379:methods*; D006801:Humans; D008628:Mercury / Q000032:analysis*; D008956:Models, Chemical
chemical_list: D000393:Air Pollutants; D008628:Mercury
keywords: Arctic; climate change; long-range transport; mercury; modelling