title: Enhanced Thermoelectric Performance of Nanostructured Bi2Te3 through Significant Phonon Scattering.
abstract: N-type Bi2Te3 nanostructures were synthesized using a solvothermal method and in turn sintered using sparking plasma sintering. The sintered n-type Bi2Te3 pellets reserved nanosized grains and showed an ultralow lattice thermal conductivity (∼0.2 W m(-1) K(-1)), which benefits from high-density small-angle grain boundaries accommodated by dislocations. Such a high phonon scattering leads an enhanced ZT of 0.88 at 400 K. This study provides an efficient method to enhance thermoelectric performance of thermoelectric nanomaterials through nanostructure engineering, making the as-prepared n-type nanostructured Bi2Te3 as a promising candidate for room-temperature thermoelectric power generation and Peltier cooling.
authors.affiliation: Materials Engineering, The University of Queensland , Brisbane, Queensland 4072, Australia.
authors.forename: Lei
authors.initials: L
authors.lastname: Yang
authors.affiliation: Materials Engineering, The University of Queensland , Brisbane, Queensland 4072, Australia.
authors.forename: Zhi-Gang
authors.initials: ZG
authors.lastname: Chen
authors.affiliation: Materials Engineering, The University of Queensland , Brisbane, Queensland 4072, Australia.
authors.forename: Min
authors.initials: M
authors.lastname: Hong
authors.affiliation: Materials Engineering, The University of Queensland , Brisbane, Queensland 4072, Australia.
authors.forename: Guang
authors.initials: G
authors.lastname: Han
authors.affiliation: Materials Engineering, The University of Queensland , Brisbane, Queensland 4072, Australia.|Centre for Microscopy and Microanalysis, The University of Queensland , Brisbane, Queensland 4072, Australia.
authors.forename: Jin
authors.initials: J
authors.lastname: Zou
keywords: Bi2Te3; enhanced thermoelectric properties; low thermal conductivity; nanostructure engineering