title: Guided Evolution of Bulk Metallic Glass Nanostructures: A Platform for Designing 3D Electrocatalytic Surfaces.
abstract: Electrochemical devices such as fuel cells, electrolyzers, lithium-air batteries, and pseudocapacitors are expected to play a major role in energy conversion/storage in the near future. Here, it is demonstrated how desirable bulk metallic glass compositions can be obtained using a combinatorial approach and it is shown that these alloys can serve as a platform technology for a wide variety of electrochemical applications through several surface modification techniques.
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.|Hydrogen and Fuel Cell Center, Nuclear and Energy Research Institute, IPEN/CNEN, SP. Av. Prof. Lineu Prestes, 2242, Cidade Universitária Lineu Prestes Cidade Universitária, São Paulo, SP, 05508-000, Brazil.
authors.forename: Gustavo
authors.initials: G
authors.lastname: Doubek
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Ryan C
authors.initials: RC
authors.lastname: Sekol
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Jinyang
authors.initials: J
authors.lastname: Li
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.
authors.forename: Won-Hee
authors.initials: WH
authors.lastname: Ryu
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.
authors.forename: Forrest S
authors.initials: FS
authors.lastname: Gittleson
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Siamak
authors.initials: S
authors.lastname: Nejati
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Eric
authors.initials: E
authors.lastname: Moy
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Candy
authors.initials: C
authors.lastname: Reid
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Marcelo
authors.initials: M
authors.lastname: Carmo
authors.affiliation: Hydrogen and Fuel Cell Center, Nuclear and Energy Research Institute, IPEN/CNEN, SP. Av. Prof. Lineu Prestes, 2242, Cidade Universitária Lineu Prestes Cidade Universitária, São Paulo, SP, 05508-000, Brazil.
authors.forename: Marcelo
authors.initials: M
authors.lastname: Linardi
authors.affiliation: Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.|Department of Mechanical Engineering and Materials Science, Yale University, New Haven, CT, 06520, USA.
authors.forename: Punnathat
authors.initials: P
authors.lastname: Bordeenithikasem
authors.affiliation: Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.|Department of Mechanical Engineering and Materials Science, Yale University, New Haven, CT, 06520, USA.
authors.forename: Emily
authors.initials: E
authors.lastname: Kinser
authors.affiliation: Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.|Department of Mechanical Engineering and Materials Science, Yale University, New Haven, CT, 06520, USA.
authors.forename: Yanhui
authors.initials: Y
authors.lastname: Liu
authors.affiliation: Center for Functional Nanomaterials, Brookhaven National Laboratory, Upton, NY, 11973, USA.
authors.forename: Xiao
authors.initials: X
authors.lastname: Tong
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Chinedum O
authors.initials: CO
authors.lastname: Osuji
authors.affiliation: Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.|Department of Mechanical Engineering and Materials Science, Yale University, New Haven, CT, 06520, USA.
authors.forename: Jan
authors.initials: J
authors.lastname: Schroers
authors.affiliation: Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: Sundeep
authors.initials: S
authors.lastname: Mukherjee
authors.affiliation: Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA.|Center for Research on Interface Structures and Phenomena, Yale University, New Haven, CT, 06520, USA.
authors.forename: André D
authors.initials: AD
authors.lastname: Taylor
keywords: bulk metallic glass; electrocatalysts; nanomaterials; pesudocapacitors; surface modification