title: (129)I record of nuclear activities in marine sediment core from Jiaozhou Bay in China.
abstract: Iodine-129 has been used as a powerful tool for environmental tracing of human nuclear activities. In this work, a sediment core collected from Jiaozhou Bay, the east coast of China, in 2002 was analyzed for (129)I to investigate the influence of human nuclear activities in this region. Significantly enhanced (129)I level was observed in upper 70 cm of the sediment core, with peak values in the layer corresponding to 1957, 1964, 1974, 1986, and after 1990. The sources of (129)I and corresponding transport processes in this region are discussed, including nuclear weapons testing at the Pacific Proving Grounds, global fallout from a large numbers of nuclear weapon tests in 1963, the climax of Chinese nuclear weapons testing in the early 1970s, the Chernobyl accident in 1986, and long-distance dispersion of European reprocessing derived (129)I. The very well (129)I records of different human nuclear activities in the sediment core illustrate the potential application of (129)I in constraining ages and sedimentation rates of the recent sediment. The releases of (129)I from the European nuclear fuel reprocessing plants at La Hague (France) and Sellafield (UK) were found to dominate the inventory of (129)I in the Chinese sediments after 1990, not only the directly atmospheric releases of these reprocessing plants, but also re-emission of marine discharged (129)I of these reprocessing plants in the highly contaminated European seas.
authors.affiliation: Xi'an AMS Center, SKLLQG, Shaanxi Key Laboratory of AMS Technology and Application, Institute of Earth Environment, CAS, Xi'an, 710061, China.
authors.forename: Yukun
authors.initials: Y
authors.lastname: Fan
authors.affiliation: Xi'an AMS Center, SKLLQG, Shaanxi Key Laboratory of AMS Technology and Application, Institute of Earth Environment, CAS, Xi'an, 710061, China. Electronic address: houxl@ieecas.cn.
authors.forename: Xiaolin
authors.initials: X
authors.lastname: Hou
authors.affiliation: Xi'an AMS Center, SKLLQG, Shaanxi Key Laboratory of AMS Technology and Application, Institute of Earth Environment, CAS, Xi'an, 710061, China.
authors.forename: Weijian
authors.initials: W
authors.lastname: Zhou
authors.affiliation: College of the Environment and Ecology, Xiamen University, Xiamen, 361005, China.
authors.forename: Guangshan
authors.initials: G
authors.lastname: Liu
mesh_terms: D061006:Bays; D002681:China; D019015:Geologic Sediments / Q000032:analysis*; D007457:Iodine Radioisotopes / Q000032:analysis*; D011834:Radiation Monitoring; D014875:Water Pollutants, Radioactive / Q000032:analysis*
chemical_list: D007457:Iodine Radioisotopes; D014875:Water Pollutants, Radioactive
keywords: Accelerator mass spectrometry; Iodine-129; Nuclear activity; Radioactivity; Sediment