title: Narrowing of the linewidth of an optical parametric oscillator by an acousto-optic modulator for the realization of mid-IR noise-immune cavity-enhanced optical heterodyne molecular spectrometry down to 10⁻¹⁰ cm⁻¹ Hz⁻¹/².
abstract: The linewidth of a singly resonant optical parametric oscillator (OPO) has been narrowed with respect to an external cavity by the use of an acousto-optic modulator (AOM). This made possible an improvement of the sensitivity of a previously realized OPO-based noise-immune cavity-enhanced optical heterodyne molecular spectrometry instrument for the 3.2 - 3.9 µm mid-infrared region by one order of magnitude. The resulting system shows a detection sensitivity for methane of 2.4 × 10(-10) cm(-1) Hz(-1∕2) and 1.3 × 10(-10) cm(-1) at 20 s, which allows for detection of both the environmentally important (13)CH(4) and CH(3)D isotopologues in atmospheric samples.
authors.forename: Thomas
authors.initials: T
authors.lastname: Hausmaninger
authors.forename: Isak
authors.initials: I
authors.lastname: Silander
authors.forename: Ove
authors.initials: O
authors.lastname: Axner