title: Tracking the photodissociation probability of D(2)(+) induced by linearly chirped laser pulses.
abstract: In the presence of linearly varying frequency chirped laser pulses, the photodissociation dynamics of D2(+) is studied theoretically after ionization of D2. As a completion of our recent work [A. Csehi et al., J. Chem. Phys. 143, 014305 (2015)], a comprehensive dependence on the pulse duration and delay time is presented in terms of total dissociation probabilities. Our numerical analysis carried out in the recently introduced light-induced conical intersection (LICI) framework clearly shows the effects of the changing position of the LICI which is induced by the frequency modulation of the chirped laser pulses. This impact is presented for positively, negatively, and zero chirped short pulses.
authors.affiliation: Department of Theoretical Physics, University of Debrecen, P.O. Box 5, H-4010 Debrecen, Hungary.
authors.forename: András
authors.initials: A
authors.lastname: Csehi
authors.affiliation: Department of Information Technology, University of Debrecen, P.O. Box 12, H-4010 Debrecen, Hungary.
authors.forename: Gábor J
authors.initials: GJ
authors.lastname: Halász
authors.affiliation: Theoretische Chemie, Physikalish-Chemisches Institut, Universität Heidelberg, H-69120 Heidelberg, Germany.
authors.forename: Lorenz S
authors.initials: LS
authors.lastname: Cederbaum
authors.affiliation: Department of Theoretical Physics, University of Debrecen, P.O. Box 5, H-4010 Debrecen, Hungary.
authors.forename: Ágnes
authors.initials: Á
authors.lastname: Vibók