title: Human health risk assessment of heavy metals in urban stormwater.
abstract: Toxic chemical pollutants such as heavy metals (HMs) are commonly present in urban stormwater. These pollutants can pose a significant risk to human health and hence a significant barrier for urban stormwater reuse. The primary aim of this study was to develop an approach for quantitatively assessing the risk to human health due to the presence of HMs in stormwater. This approach will lead to informed decision making in relation to risk management of urban stormwater reuse, enabling efficient implementation of appropriate treatment strategies. In this study, risks to human health from heavy metals were assessed as hazard index (HI) and quantified as a function of traffic and land use related parameters. Traffic and land use are the primary factors influencing heavy metal loads in the urban environment. The risks posed by heavy metals associated with total solids and fine solids (<150μm) were considered to represent the maximum and minimum risk levels, respectively. The study outcomes confirmed that Cr, Mn and Pb pose the highest risks, although these elements are generally present in low concentrations. The study also found that even though the presence of a single heavy metal does not pose a significant risk, the presence of multiple heavy metals could be detrimental to human health. These findings suggest that stormwater guidelines should consider the combined risk from multiple heavy metals rather than the threshold concentration of an individual species. Furthermore, it was found that risk to human health from heavy metals in stormwater is significantly influenced by traffic volume and the risk associated with stormwater from industrial areas is generally higher than that from commercial and residential areas.
authors.affiliation: Science and Engineering Faculty, Queensland University of Technology (QUT), GPO Box 2434, Brisbane 4001, Queensland, Australia.
authors.forename: Yukun
authors.initials: Y
authors.lastname: Ma
authors.affiliation: Science and Engineering Faculty, Queensland University of Technology (QUT), GPO Box 2434, Brisbane 4001, Queensland, Australia.
authors.forename: Prasanna
authors.initials: P
authors.lastname: Egodawatta
authors.affiliation: Science and Engineering Faculty, Queensland University of Technology (QUT), GPO Box 2434, Brisbane 4001, Queensland, Australia.
authors.forename: James
authors.initials: J
authors.lastname: McGree
authors.affiliation: College of Chemistry and Environmental Engineering, Shenzhen University, 518060 Shenzhen, China.
authors.forename: An
authors.initials: A
authors.lastname: Liu
authors.affiliation: Science and Engineering Faculty, Queensland University of Technology (QUT), GPO Box 2434, Brisbane 4001, Queensland, Australia. Electronic address: a.goonetilleke@qut.edu.au.
authors.forename: Ashantha
authors.initials: A
authors.lastname: Goonetilleke
mesh_terms: D002947:Cities; D004781:Environmental Exposure / Q000706:statistics & numerical data*; D006801:Humans; D019216:Metals, Heavy / Q000032:analysis*; D011891:Rain; D018570:Risk Assessment; D062065:Wastewater / Q000737:chemistry; D014874:Water Pollutants, Chemical / Q000032:analysis*
chemical_list: D019216:Metals, Heavy; D062065:Wastewater; D014874:Water Pollutants, Chemical
keywords: Hazard index; Heavy metals; Risk assessment; Stormwater pollutant processes; Stormwater quality