title: Uniaxial ferroelectric quantum criticality in multiferroic hexaferrites BaFe12O19 and SrFe12O19.
abstract: BaFe12O19 is a popular M-type hexaferrite with a Néel temperature of 720 K and is of enormous commercial value ($3 billion/year). It is an incipient ferroelectric with an expected ferroelectric phase transition extrapolated to lie at 6 K but suppressed due to quantum fluctuations. The theory of quantum criticality for such uniaxial ferroelectrics predicts that the temperature dependence of the electric susceptibility χ diverges as 1/T(3), in contrast to the 1/T(2) dependence found in pseudo-cubic materials such as SrTiO3 or KTaO3. In this paper we present evidence of the susceptibility varying as 1/T(3), i.e. with a critical exponent γ = 3. In general γ = (d + z - 2)/z, where the dynamical exponent for a ferroelectric z = 1 and the dimension is increased by 1 from deff = 3 + z to deff = 4 + z due to the effect of long-range dipole interactions in uniaxial as opposed to multiaxial ferroelectrics. The electric susceptibility of the incipient ferroelectric SrFe12O19, which is slightly further from the quantum phase transition is also found to vary as 1/T(3).
authors.affiliation: Cavendish Laboratory, Cambridge University, J. J. Thomson Avenue, Cambridge, CB3 0HE, United Kingdom.|Centro Brasileiro de Pesquisas Físicas, Rua Dr Xavier Sigaud 150, Urca, Rio de Janeiro, 22290-180, Brazil.
authors.forename: S E
authors.initials: SE
authors.lastname: Rowley
authors.affiliation: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
authors.forename: Yi-Sheng
authors.initials: YS
authors.lastname: Chai
authors.affiliation: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
authors.forename: Shi-Peng
authors.initials: SP
authors.lastname: Shen
authors.affiliation: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
authors.forename: Young
authors.initials: Y
authors.lastname: Sun
authors.affiliation: Cavendish Laboratory, Cambridge University, J. J. Thomson Avenue, Cambridge, CB3 0HE, United Kingdom.
authors.forename: A T
authors.initials: AT
authors.lastname: Jones
authors.affiliation: IMEM-CNR, Parco Area delle Scienze 37/A, 43124 Parma, Italy.
authors.forename: B E
authors.initials: BE
authors.lastname: Watts
authors.affiliation: Cavendish Laboratory, Cambridge University, J. J. Thomson Avenue, Cambridge, CB3 0HE, United Kingdom.|Schools of Chemistry and of Physics and Astronomy, St. Andrews University, St. Andrews, Fife, KY16 9ST, United Kingdom.
authors.forename: J F
authors.initials: JF
authors.lastname: Scott