High-Performance Inkjet-Printed Indium-Gallium-Zinc-Oxide Transistors Enabled by Embedded, Chemically Stable Graphene Electrodes.
Recent developments in solution-processed amorphous oxide semiconductors have established indium-gallium-zinc-oxide (IGZO) as a promising candidate for printed electronics. A key challenge for this vision is the integration of IGZO thin-film transistor (TFT) channels with compatible source/drain electrodes using low-temperature, solution-phase patterning methods. Here we demonstrate the suitability of inkjet-printed graphene electrodes for this purpose. In contrast to common inkjet-printed silver-based conductive inks, graphene provides a chemically stable electrode-channel interface. Furthermore, by embedding the graphene electrode between two consecutive IGZO printing passes, high-performance IGZO TFTs are achieved with an electron mobility of ∼6 cm(2)/V·s and current on/off ratio of ∼10(5). The resulting printed devices exhibit robust stability to aging in ambient as well as excellent resilience to thermal stress, thereby offering a promising platform for future printed electronics applications.
Department of Materials Science and Engineering and the Materials Research Center, Northwestern University , Evanston, Illinois 60208, United States.
Ethan B
EB
Secor
Department of Chemistry and the Materials Research Center, Northwestern University , Evanston, Illinois 60208, United States.
Jeremy
J
Smith
Department of Materials Science and Engineering and the Materials Research Center, Northwestern University , Evanston, Illinois 60208, United States.|Department of Chemistry and the Materials Research Center, Northwestern University , Evanston, Illinois 60208, United States.
Tobin J
TJ
Marks
Department of Materials Science and Engineering and the Materials Research Center, Northwestern University , Evanston, Illinois 60208, United States.|Department of Chemistry and the Materials Research Center, Northwestern University , Evanston, Illinois 60208, United States.|Department of Electrical Engineering and Computer Science, Northwestern University , Evanston, Illinois 60208, United States.
Mark C
MC
Hersam
amorphous oxide semiconductor; graphene; inkjet printing; printed electronics; stability; thin-film transistor