title: Intraurban Variation of Fine Particle Elemental Concentrations in New York City.
abstract: Few past studies have collected and analyzed within-city variation of fine particulate matter (PM2.5) elements. We developed land-use regression (LUR) models to characterize spatial variation of 15 PM2.5 elements collected at 150 street-level locations in New York City during December 2008-November 2009: aluminum, bromine, calcium, copper, iron, potassium, manganese, sodium, nickel, lead, sulfur, silicon, titanium, vanadium, and zinc. Summer- and winter-only data available at 99 locations in the subsequent 3 years, up to November 2012, were analyzed to examine variation of LUR results across years. Spatial variation of each element was modeled in LUR including six major emission indicators: boilers burning residual oil; traffic density; industrial structures; construction/demolition (these four indicators in buffers of 50 to 1000 m), commercial cooking based on a dispersion model; and ship traffic based on inverse distance to navigation path weighted by associated port berth volume. All the elements except sodium were associated with at least one source, with R(2) ranging from 0.2 to 0.8. Strong source-element associations, persistent across years, were found for residual oil burning (nickel, zinc), near-road traffic (copper, iron, and titanium), and ship traffic (vanadium). These emission source indicators were also significant and consistent predictors of PM2.5 concentrations across years.
authors.affiliation: Bureau of Environmental Surveillance and Policy, New York City Department of Health and Mental Hygiene , New York, New York 10013, United States.
authors.forename: Kazuhiko
authors.initials: K
authors.lastname: Ito
authors.affiliation: Bureau of Environmental Surveillance and Policy, New York City Department of Health and Mental Hygiene , New York, New York 10013, United States.
authors.forename: Sarah
authors.initials: S
authors.lastname: Johnson
authors.affiliation: Bureau of Environmental Surveillance and Policy, New York City Department of Health and Mental Hygiene , New York, New York 10013, United States.
authors.forename: Iyad
authors.initials: I
authors.lastname: Kheirbek
authors.affiliation: Department of Environmental and Occupational Health, University of Pittsburgh, Graduate School of Public Health , Pittsburgh, Pennsylvania 15219, United States.
authors.forename: Jane
authors.initials: J
authors.lastname: Clougherty
authors.affiliation: Bureau of Environmental Surveillance and Policy, New York City Department of Health and Mental Hygiene , New York, New York 10013, United States.
authors.forename: Grant
authors.initials: G
authors.lastname: Pezeshki
authors.affiliation: ZevRoss Spatial Analysis , Ithaca, New York 14850, United States.
authors.forename: Zev
authors.initials: Z
authors.lastname: Ross
authors.affiliation: Barry Commoner Center for Health and the Environment, Queens College, City University of New York , Flushing, New York, New York 11367, United States.
authors.forename: Holger
authors.initials: H
authors.lastname: Eisl
authors.affiliation: Bureau of Environmental Surveillance and Policy, New York City Department of Health and Mental Hygiene , New York, New York 10013, United States.
authors.forename: Thomas D
authors.initials: TD
authors.lastname: Matte
mesh_terms: D000393:Air Pollutants; D002947:Cities; D008962:Models, Theoretical; D009519:New York City; D052638:Particulate Matter; D014639:Vanadium
chemical_list: D000393:Air Pollutants; D052638:Particulate Matter; D014639:Vanadium