Color-tunable emission of quantum dots via strong exciton-plasmon coupling in nanoporous gold structure at room temperature.
We experimentally demonstrate the color-tunable emission of CdTe quantum dots (QDs) enabled by strongly coupling the QDs to the nanoporous gold (NPG) structure at room temperature. By manipulating the concentrations of the QDs or the excitation flux of the laser, the coupling strength between the excitons in QDs and the plasmons in NPG is controlled, resulting in a large Rabi splitting at the magnitude of hundreds of meV and a photoluminescence (PL) tuning distinguishable by the naked eye. In addition, such large PL tuning is enabled not only for the strong coupling occurring on resonance but also off resonance. We believe that our study offers a new approach towards designing and fabricating novel opto-electronic devices where dynamical and large spectral tuning of QD PL emission is desired.
X
X
Zhao
L
L
Chen
J
J
Chen
W
W
Shi
F
F
Liu