title: Hierarchical silicalite-1 octahedra comprising highly-branched orthogonally-stacked nanoplates as efficient catalysts for vapor-phase Beckmann rearrangement.
abstract: A triblock structure-directing agent was designed to synthesize hierarchical silicalite-1 octahedra comprising highly-branched, orthogonally-stacked and self-pillared nanoplates that exhibited excellent and stable activity for the vapor-phase Beckmann rearrangement of cyclic oximes and high lactam selectivity.
authors.affiliation: Department of Chemistry, National Tsing Hua University, Hsinchu 30013, Taiwan. cmyang@mx.nthu.edu.tw.
authors.forename: Albert
authors.initials: A
authors.lastname: Chang
authors.affiliation: Department of Chemistry, National Tsing Hua University, Hsinchu 30013, Taiwan. cmyang@mx.nthu.edu.tw.
authors.forename: Hsu-Ming
authors.initials: HM
authors.lastname: Hsiao
authors.affiliation: Department of Chemistry, National Tsing Hua University, Hsinchu 30013, Taiwan. cmyang@mx.nthu.edu.tw.
authors.forename: Tsai-Hsiu
authors.initials: TH
authors.lastname: Chen
authors.affiliation: Center for Condensed Matter Sciences, National Taiwan University, Taipei 10617, Taiwan.
authors.forename: Ming-Wen
authors.initials: MW
authors.lastname: Chu
authors.affiliation: Department of Chemistry, National Tsing Hua University, Hsinchu 30013, Taiwan. cmyang@mx.nthu.edu.tw and Frontier Research Center on Fundamental and Applied Sciences of Matters, National Tsing Hua University, Hsinchu 30013, Taiwan.
authors.forename: Chia-Min
authors.initials: CM
authors.lastname: Yang