title: A Novel Lithiated Silicon-Sulfur Battery Exploiting an Optimized Solid-Like Electrolyte to Enhance Safety and Cycle Life.
abstract: Anovel lithiated Si-S battery exploiting an optimized solid-like electrolyte is presented. This electrolyte is fabricated by integrating ether-based liquid electrolyte with SiO2hollow nanosphere layer to suppress the shuttle effect and fluoroethylene carbonate additive to optimize the anodic solid electrolyte interface. The prepared lithiated Si-S batteries exhibit enhanced cycle life, low flammability, and strong recovery ability against short-circuit.
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.|State Key Laboratory of New Ceramics and Fine Processing, and Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, P. R. China.
authors.forename: Dong
authors.initials: D
authors.lastname: Zhou
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.|State Key Laboratory of New Ceramics and Fine Processing, and Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, P. R. China.
authors.forename: Ming
authors.initials: M
authors.lastname: Liu
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.|State Key Laboratory of New Ceramics and Fine Processing, and Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, P. R. China.
authors.forename: Qinbai
authors.initials: Q
authors.lastname: Yun
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.|State Key Laboratory of New Ceramics and Fine Processing, and Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, P. R. China.
authors.forename: Xia
authors.initials: X
authors.lastname: Wang
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.
authors.forename: Yan-Bing
authors.initials: YB
authors.lastname: He
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.
authors.forename: Baohua
authors.initials: B
authors.lastname: Li
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.
authors.forename: Quan-Hong
authors.initials: QH
authors.lastname: Yang
authors.affiliation: State Key Laboratory of New Ceramics and Fine Processing, and Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, P. R. China.
authors.forename: Qiang
authors.initials: Q
authors.lastname: Cai
authors.affiliation: National Local Joint Engineering Laboratory of Carbon Functional Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, 518055, P. R. China.|State Key Laboratory of New Ceramics and Fine Processing, and Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, P. R. China.
authors.forename: Feiyu
authors.initials: F
authors.lastname: Kang
keywords: SiO2 hollow nanospheres; fluoroethylene carbonate; lithiated silicon-sulfur batteries; optimized solid-like electrolytes; safety