title: Multifunctional Carbon-Based Metal-Free Electrocatalysts for Simultaneous Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution.
abstract: Rationally designed N, S co-doped graphitic sheets with stereoscopic holes (SHG) act as effective tri-functional catalysts for the oxygen reduction reaction, hydrogen evolution reaction, and oxygen evolution reaction, simultaneously. The multifunctional electrocatalytic activities originate from a synergistic effect of the N, S heteroatom doping and unique SHG architecture, which provide a large surface area and efficient pathways for electron and electrolyte/reactant transports.
authors.affiliation: Center of Advanced Science and Engineering for Carbon (Case 4carbon), Department of Macromolecular Science and Engineering, Case Western Reserve University, 10900 Euclid Avenue, Cleveland, OH, 44106, USA.
authors.forename: Chuangang
authors.initials: C
authors.lastname: Hu
authors.affiliation: Center of Advanced Science and Engineering for Carbon (Case 4carbon), Department of Macromolecular Science and Engineering, Case Western Reserve University, 10900 Euclid Avenue, Cleveland, OH, 44106, USA.
authors.forename: Liming
authors.initials: L
authors.lastname: Dai
keywords: hydrogen evolution reaction (HER); multifunctional metal-free catalyst; oxygen evolution reaction (OER); oxygen reduction reaction (ORR); water splitting