title: Exploiting Vibrational Strong Coupling to Make an Optical Parametric Oscillator Out of a Raman Laser.
abstract: When the collective coupling of the rovibrational states in organic molecules and confined electromagnetic modes is sufficiently strong, the system enters into vibrational strong coupling, leading to the formation of hybrid light-matter quasiparticles. In this Letter, we demonstrate theoretically how this hybridization in combination with stimulated Raman scattering can be utilized to widen the capabilities of Raman laser devices. We explore the conditions under which the lasing threshold can be diminished and the system can be transformed into an optical parametric oscillator. Finally, we show how the dramatic reduction of the many final molecular states into two collective excitations can be used to create an all-optical switch with output in the midinfrared.
authors.affiliation: Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Madrid, Spain.
authors.forename: Javier
authors.initials: J
authors.lastname: Del Pino
authors.affiliation: Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Madrid, Spain.|Donostia International Physics Center (DIPC), E-20018 Donostia/San Sebastián, Spain.
authors.forename: Francisco J
authors.initials: FJ
authors.lastname: Garcia-Vidal
authors.affiliation: Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Madrid, Spain.
authors.forename: Johannes
authors.initials: J
authors.lastname: Feist