Revisiting the fission track method for the analysis of particles in safeguards environmental samples.
This paper details an improved approach to environmental particle analysis for safeguards by means of a combination of an upgraded version of the so-called fission track method with state-of-the-art microscope and microprobe techniques. Improvements to the fission track method comprise a novel sample assembly, the automation of several of its steps and the extensive use of correlative microscopy. This is followed by an automated isolation of particles-of-interest by means of laser micro-dissection (LMD) and their collection onto a harvester for transfer to other micro-analytical instruments for further analysis. The samples examined in this contribution were analysed for their nuclear material signatures, in particular the presence of uranium isotopes. The length of a single analysis cycle herewith was reduced to 12 days.
TU Wien, Institute of Chemical and Analytical Technologies, Getreidemarkt 9/164, 1060 Vienna, Austria. Electronic address: naida.dzigal@student.tuwien.ac.at.
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Dzigal
International Atomic Energy Agency, Wagramerstrasse 1, 1220 Vienna, Austria. Electronic address: e.chinea-cano@iaea.org.
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Chinea-Cano
International Atomic Energy Agency, Wagramerstrasse 1, 1220 Vienna, Austria.
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Walsh
TU Wien, Institute of Chemical and Analytical Technologies, Getreidemarkt 9/164, 1060 Vienna, Austria.
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Limbeck
Correlative microscopy; Environmental swipe samples; Fission track; LA-ICP-MS; LMD; Safeguards