title: Enhanced Performance of a Self-Powered Organic/Inorganic Photodetector by Pyro-Phototronic and Piezo-Phototronic Effects.
abstract: Self-powered photodetectors (PDs) have long been realized by utilizing photovoltaic effect and their performances can be effectively enhanced by introducing the piezo-phototronic effect. Recently, a novel pyro-phototronic effect is invented as an alternative approach for performance enhancement of self-powered PDs. Here, a self-powered organic/inorganic PD is demonstrated and the influences of externally applied strain on the pyro-phototronic and the photovoltaic effects are thoroughly investigated. Under 325 nm 2.30 mW cm-2UV illumination and at a -0.45% compressive strain, the PD's photocurrent is dramatically enhanced from ≈14.5 to ≈103 nA by combining the pyro-phototronic and piezo-phototronic effects together, showing a significant improvement of over 600%. Theoretical simulations have been carried out via the finite element method to propose the underlying working mechanism. Moreover, the pyro-phototronic effect can be introduced by applying a -0.45% compressive strain to greatly enhance the PD's response to 442 nm illumination, including photocurrent, rise time, and fall time. This work provides in-depth understandings about the pyro-phototronic and the piezo-phototronic effects on the performances of self-powered PD to light sources with different wavelengths and indicates huge potential of these two effects in optoelectronic devices.
authors.affiliation: School of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049, China.|School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
authors.forename: Wenbo
authors.initials: W
authors.lastname: Peng
authors.affiliation: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
authors.forename: Xingfu
authors.initials: X
authors.lastname: Wang
authors.affiliation: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
authors.forename: Ruomeng
authors.initials: R
authors.lastname: Yu
authors.affiliation: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
authors.forename: Yejing
authors.initials: Y
authors.lastname: Dai
authors.affiliation: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
authors.forename: Haiyang
authors.initials: H
authors.lastname: Zou
authors.affiliation: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
authors.forename: Aurelia C
authors.initials: AC
authors.lastname: Wang
authors.affiliation: School of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049, China.
authors.forename: Yongning
authors.initials: Y
authors.lastname: He
authors.affiliation: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332, USA.|Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of Sciences, Beijing, 100083, China.
authors.forename: Zhong Lin
authors.initials: ZL
authors.lastname: Wang
keywords: ZnO; photodetectors; piezo-phototronic effect; pyro-phototronic effect